The main difference is that you're using a Take Folder and Take Folders don't automatically add to the Comp when you extend their left side like that. Nor can you crossfade Take Folders. You can open the Take Folder and Swipe the beginning of the active Take to the left, but that still may leave an audible click between the Folders.
One good way to accomplish this would be to Flatten the Take Folders without merging so you can still move things around. To do this, left click the Comp indicator, which in your case is the "B" next to "GTR Interlude: Comp C" and click Flatten. Be aware that this will get rid of the Take Folder.
Personally, I would prefer turning all the Take Folders on that track to Track Alternatives at this point for this exact reason. It preserves all your Comps and Takes while allowing you to move, expand, and crossfade individual regions on the Active Track Alternative.